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Flood frequency analysis (FFA) entails the estimation of the upper tail of a probability density function (PDF) of annual peak flows obtained from either the annual maximum series or partial duration series. In hydrological practice, the properties of various methods of upper quantiles estimation are identified with the case of known population distribution function. In reality, the assumed hypothetical model differs from the true one and one cannot assess the magnitude of error caused by model misspecification in respect to any estimated statistics. The opinion about the accuracy of the methods of upper quantiles estimation formed from the case of known population distribution function is upheld. The above-mentioned issue is the subject of the paper. The accuracy of large quantile assessments obtained from the four estimation methods is compared to two-parameter log-normal and log-Gumbel distributions and their three-parameter counterparts, i.e., three-parameter log-normal and GEV distributions. The cases of true and false hypothetical models are considered. The accuracy of flood quantile estimates depends on the sample size, the distribution type (both true and hypothetical), and strongly depends on the estimation method. In particular, the maximum likelihood method loses its advantageous properties in case of model misspecification.